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Figures of the Article
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(a) XRD patterns of as-milled Li2−2xMn1−xZrxCl4. (b) Partial enlarged image of (a).
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XRD patterns of the 350 °C-annealed Li2−2xMn1−xZrxCl4 powder samples.
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Conductivity of LMZC5 under different processing conditions. (a, b) Nyquist plots of the as-milled (a) and 350 °C-annealed (b) LMZC5 at 25 °C. (c, d) Chronoamperometry results for the as-milled (c) and 350 °C-annealed (d) LMZC5 at 25 °C with a voltage step of 1 V.
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Conductivity and activation energy evolution upon Zr4+ substitution. (a) Arrhenius plots of Li+ conductivity for as-milled Li2−2xMn1−xZrxCl4. (b) Ionic conductivities at 25 °C and activation energies of as-milled Li2-2xMn1-xZrxCl4.
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Thermodynamic equilibrium voltage profiles and the phase equilibria for LMZC5 based on DFT calculations.
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LSV curves of the Li/Li6PS5Cl-LMZC5/LMZC5+C cell at 0.1 mV∙s−1. The measurements were conducted at room temperature. (a) 0–3.1 V. (b) 3–5 V.
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Electrochemical performance of the Li-In/Li6PS5Cl-LIC/LMZC5 cell at 25 °C. (a) Charge and discharge profiles at 0.1 C. (b) Rate performance. (c) Long-term cycling performance at 0.1 C.
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(a) Ex situ XRD patterns of LMZC5 at different depths of discharge (DoDs). The DoD of each XRD pattern is indicated in (b). (b) The initial discharge profile at 0.1 C, with the DoD for each XRD pattern in (a) indicated.
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