High-sensitivity double-quantum magnetometry in diamond via quantum control

High-fidelity quantum operation of qubits plays an important role in magnetometry based on nitrogen-vacancy (NV) centers in diamonds. However, the nontrivial spin-spin coupling of the NV center decreases signal contrast and sensitivity. Here, we overcome this limitation by exploiting the amplitude modulation of microwaves, which allows us to perfectly detect magnetic signals at low fields. Compared with the traditional double-quantum sensing protocol, the full contrast of the detection signal was recovered, and the sensitivity was enhanced three times in the experiment. Our method is applicable to a wide range of sensing tasks, such as temperature, strain, and electric field.